Joshua DiGangi

and 13 more

Southeast Asian biomass burning is a major pollutant source that contributes to poor air quality throughout the region. Thus, understanding these emissions is critical for predicting and mitigating their health impacts. While many studies have reported ground-based and satellite measurements, airborne measurements at a regional scale capable of tying the two together have not been common. The 2019 Cloud, Aerosol and Monsoon Processes Philippines Experiment (CAMP2Ex) field project examined Southeast Asian regional sources and their effects on aerosol/cloud interactions using a combination of airborne, shipboard, and ground-based measurements. These flights sampled a variety of airmass sources over the Philippine, South China, and Sulu seas during both the southwest monsoon and monsoon transition periods. Measurements during CAMP2Ex provide a unique opportunity to investigate how these transported and local emissions affected air quality trends and airmass chemical composition. We present correlated airborne in situ enhancement ratios of CH4 to CO, using them to identify source regimes of either high urban or biomass burning influence as well as urban regimes with different emission factors. Combined with backtrajectory analysis using HYSPLIT, source regimes were examined for differences in ozone, reactive nitrogen, and aerosol chemical composition. While observed O3/CO enhancement ratios remain constant for differing urban source regimes, NOy/CO ratios varied across these regimes. For biomass burning sources, O3/CO enhancement ratios are observed to be lower than previously reported by measurements in the region.

Melissa Yang

and 52 more

The 2020 COVID-19 pandemic provided a unique opportunity to sample atmospheric gases during a period of very low industrial/human activity. Over 1000 Whole Air Samples were collected in over 30 cities and towns across the United States from April through July 2020 as part of the NASA Student Airborne Research Program (SARP). Sample locations leveraged the geographic distribution across the United States of the undergraduate and graduate students, faculty, and NASA personnel associated with the internship program (44 people total). Each person collected approximately 24 air samples in their city/town with the goal of characterizing local emissions with time during the pandemic. Samples were collected in 2-Liter stainless steel evacuated canisters at approximately 2 meters above ground level. The canisters were shipped to the Rowland/Blake Laboratory at the University of California Irvine and analyzed for methane, carbon dioxide, carbon monoxide, non-methane hydrocarbons, and halocarbons using the gas chromatographic system described in Colman et al. (2001) and Barletta et al. (2002). Initial samples collected in April coincided with the peak of stay-at-home/social distancing orders across most of the United States while samples collected later in the spring and early summer reflect the easing of these measures in most locations. Overall trends in emissions with time across the United States during the pandemic (in several large metro areas as well as rural locations) will be discussed.