Changes in the concentration of greenhouse gases within the atmosphere lead to changes in radiative fluxes throughout the atmosphere. The value of this change, called the instantaneous radiative forcing, varies across climate models, due partly to differences in the distribution of clouds, humidity, and temperature across models, and partly due to errors introduced by approximate treatments of radiative transfer. This paper describes an experiment within the Radiative Forcing Model Intercomparision Project that uses benchmark calculations made with line-by-line models to identify parameterization error in the representation of absorption and emission by greenhouse gases. The clear-sky instantaneous forcing by greenhouse gases to which the world has been subject is computed using a set of 100 profiles, selected from a re-analysis of present-day conditions, that represent the global annual mean forcing with sampling errors of less than 0.01 \si{\watt\per\square\meter}. Six contributing line-by-line models agree in their estimate of this forcing to within 0.025 \si{\watt\per\square\meter} while even recently-developed parameterizations have typical errors four or more times larger, suggesting both that the samples reveal true differences among line-by-line models and that parameterization error will be readily resolved. Agreement among line-by-line models is better in the longwave than in the shortwave where differing treatments of the water vapor vapor continuum affect estimates of forcing by carbon dioxide and methane. The impacts of clouds on instantaneous radiative forcing are roughly estimated, as are adjustments due to stratospheric temperature change. Adjustments are large only for ozone and for carbon dioxide, for which stratospheric cooling introduces modest non-linearity.

This paper describes the initial implementation of a new toolbox that seeks to balance accuracy, efficiency, and flexibility in radiation calculations for dynamical models. The toolbox consists of two related code bases: Radiative Transfer for Energetics (RTE), which computes fluxes given a radiative transfer problem defined in terms of optical properties, boundary conditions and source functions, and RRTM for GCM applications - Parallel (RRTMGP), which combines data and algorithms to map a physical description of the gaseous atmosphere into such a radiative transfer problem. The toolbox is an implementation of well-established ideas, including the use of a k-distribution to represent the spectral variation of absorption by gases and the use of two-stream, plane-parallel methods for solving the radiative transfer equation. The focus is instead on accuracy, by basing the k-distribution on state-of-the-art spectroscopy, and on the sometimes-conflicting goals of flexibility and efficiency. Flexibility is facilitated by making extensive use of computational objects encompassing code and data, the latter provisioned at run time and potentially tailored to specific problems. The computational objects provide robust access to a set of high-efficiency computational kernels that can be adapted to new computational environments. Accuracy is obtained by careful choice of algorithms and through tuning and validation of the k-distribution against benchmark calculations. Flexibility with respect to the host model implies user responsibility for maps between clouds and aerosols and the radiative transfer problem, although comprehensive examples are provided for clouds.

The science guiding the \EURECA campaign and its measurements are presented. \EURECA comprised roughly five weeks of measurements in the downstream winter trades of the North Atlantic — eastward and south-eastward of Barbados. Through its ability to characterize processes operating across a wide range of scales, \EURECA marked a turning point in our ability to observationally study factors influencing clouds in the trades, how they will respond to warming, and their link to other components of the earth system, such as upper-ocean processes or, or the life-cycle of particulate matter. This characterization was made possible by thousands (2500) of sondes distributed to measure circulations on meso (200 km) and larger (500 km) scales, roughly four hundred hours of flight time by four heavily instrumented research aircraft, four global-ocean class research vessels, an advanced ground-based cloud observatory, a flotilla of autonomous or tethered measurement devices operating in the upper ocean (nearly 10000 profiles), lower atmosphere (continuous profiling), and along the air-sea interface, a network of water stable isotopologue measurements, complemented by special programmes of satellite remote sensing and modeling with a new generation of weather/climate models. In addition to providing an outline of the novel measurements and their composition into a unified and coordinated campaign, the six distinct scientific facets that \EURECA explored — from Brazil Ring Current Eddies to turbulence induced clustering of cloud droplets and its influence on warm-rain formation — are presented along with an overview \EURECA’s outreach activities, environmental impact, and guidelines for scientific practice.