The Atmospheric Carbon and Transport (ACT) – America NASA Earth Venture Suborbital Mission set out to improve regional atmospheric greenhouse gas (GHG) inversions by exploring the intersection of the strong GHG fluxes and vigorous atmospheric transport that occurs within the midlatitudes. Two research aircraft instrumented with remote and in situ sensors to measure GHG mole fractions, associated trace gases, and atmospheric state variables collected 1140.7 flight hours of research data, distributed across 305 individual aircraft sorties, coordinated within 121 research flight days, and spanning five, six-week seasonal flight campaigns in the central and eastern United States. Flights sampled 31 synoptic sequences, including fair weather and frontal conditions, at altitudes ranging from the atmospheric boundary layer to the upper free troposphere. The observations were complemented with global and regional GHG flux and transport model ensembles. We found that midlatitude weather systems contain large spatial gradients in GHG mole fractions, in patterns that were consistent as a function of season and altitude. We attribute these patterns to a combination of regional terrestrial fluxes and inflow from the continental boundaries. These observations, when segregated according to altitude and air mass, provide a variety of quantitative insights into the realism of regional CO2 and CH4 fluxes and atmospheric GHG transport realizations. The ACT-America data set and ensemble modeling methods provide benchmarks for the development of atmospheric inversion systems. As global and regional atmospheric inversions incorporate ACT-America’s findings and methods, we anticipate these systems will produce increasingly accurate and precise sub-continental GHG flux estimates.

The ACT-America project is a NASA Earth Venture Suborbital-2 mission designed to study the transport and fluxes of greenhouse gases. The open and freely available ACT-America datasets provide airborne in-situ measurements of atmospheric carbon dioxide, methane, trace gases, aerosols, clouds, and meteorological properties, airborne remote sensing measurements of aerosol backscatter, atmospheric boundary layer height and columnar content of atmospheric carbon dioxide, tower-based measurements, and modeled atmospheric mole fractions and regional carbon fluxes of greenhouse gases over the Central and Eastern United States. We conducted 121 research flights during five campaigns in four seasons during 2016-2019 over three regions of the US (Mid-Atlantic, Midwest and South) using two NASA research aircraft (B-200 and C-130). We performed three flight patterns (fair weather, frontal crossings, and OCO-2 underflights) and collected more than 1,140 hours of airborne measurements via level-leg flights in the atmospheric boundary layer, lower, and upper free troposphere and vertical profiles spanning these altitudes. We also merged various airborne in-situ measurements onto a common standard sampling interval, which brings coherence to the data, creates geolocated data products, and makes it much easier for the users to perform holistic analysis of the ACT-America data products. Here, we report on detailed information of datasets collected, and the workflow for datasets including storage and processing of the quality controlled and quality assured harmonized observations, and their archival and formatting for users. Finally, we provide some important information on the dissemination of data products including metadata and highlights of applications of datasets for future investigations.

To check the accuracy of column-average dry air CO2 mole fractions (“XCO2”) retrieved from Orbiting Carbon Overvatory (OCO-2) data, a similar quantity has been measured from the Multi-functional Fiber Laser Lidar (MFLL) aboard aircraft flying underneath OCO-2 as part of the Atmospheric Carbon and Transport (ACT)-America flight campaigns. Here we do a lagged correlation analysis of these MFLL-OCO-2 column CO2 differences and find that their correlation spectrum falls off rapidly at along-track separation distances of under 10 km, with a correlation length scale of about 10 km, and less rapidly at longer separation distances, with a correlation length scale of about 20 km. The OCO-2 satellite takes many CO2 measurements with small (∼3 km^2) fields of view (FOVs) in a thin (~10 km wide) swath running parallel to its orbit: up to 24 separate FOVs may be obtained per second (across a ∼6.75 km distance on the ground), though clouds, aerosols, and other factors cause considerable data dropout. Errors in the CO2 retrieval method have long been thought to be correlated at these fine scales, and methods to account for these when assimilating these data into 10 top-down atmospheric CO2 flux inversions have been developed. A common approach has been to average the data at coarser scales (e.g., in 10-second-long bins) along-track, then assign an uncertainty to the averaged value that accounts for the error correlations. Here we outline the methods used up to now for computing these 10-second averages and their uncertainties, including the constant-correlation-with-distance error model currently being used to summarize the OCO-2 version 9 XCO2 retrievals as part of the OCO-2 flux inversion model intercomparison project. We then derive a new one-dimensional error model using correlations that decay exponentially with separation distance, apply this model to the OCO-2 data using the correlation length scales derived from the MFLL-OCO-2 differences, and compare the results (for both the average and its uncertainty) to those given by the current constant-correlation error model. To implement this new model, the data are averaged first across 2-second spans, to collapse the cross-track distribution of the real data onto the 1-D path assumed by the new model. A small percentage of the data that cause non-physical negative averaging weights in the model are thrown out. The correlation lengths over the ocean, which the land-based MFLL data do not clarify, are assumed to be twice those over the land. The new correlation model gives 10-second XCO2 averages that are only a few tenths of a ppm different from the constant-correlation model. […] Finally, we show how our 1-D exponential error correlation model may be used to account for correlations in those inversion methods that choose to assimilate each XCO2 retrieval individually, and to account for correlations between separate 10-second averages when these are assimilated instead.