Top-down estimates of CO2 fluxes are typically constrained by either surface-based or space-based CO2 observations. Both of these measurement types have spatial and temporal gaps in observational coverage that can lead to biases in inferred fluxes. Assimilating both surface-based and space-based measurements concurrently in a flux inversion framework improves observational coverage and reduces sampling biases. This study examines the consistency of flux constraints provided by these different observations and the potential to combine them by performing a series of six-year (2010–2015) CO2 flux inversions. Flux inversions are performed assimilating surface-based measurements from the in situ and flask network, measurements from the Total Carbon Column Observing Network (TCCON), and space-based measurements from the Greenhouse Gases Observing Satellite (GOSAT), or all three datasets combined. Combining the datasets results in more precise flux estimates for sub-continental regions relative to any of the datasets alone. Combining the datasets also improves the accuracy of the posterior fluxes, based on reduced root-mean-square differences between posterior-flux-simulated CO2 and aircraft-based CO2 over midlatitude regions (0.35–0.50~ppm) in comparison to GOSAT (0.39–0.57~ppm), TCCON (0.52–0.63~ppm), or in situ and flask measurements (0.45–0.53~ppm) alone. These results suggest that surface-based and GOSAT measurements give complementary constraints on CO2 fluxes in the northern extratropics and can be combined in flux inversions to improve observational coverage. This stands in contrast with many earlier attempts to combine these datasets and suggests that improvements in the NASA Atmospheric CO2 Observations from Space (ACOS) retrieval algorithm have significantly improved the consistency of space-based and surface-based flux constraints.

Shyno Susan John

and 3 more

Fire is an essential global phenomenon that existed soon after the appearance of terrestrial plants and is vital for the regeneration of the plant species. Human activities have contributed to a changing climate and impacted fire regimes, resulting in more intense, frequent and severe fires. In particular, the 2019-20 bushfires in south-eastern Australia were unprecedented in their extent and intensity. However, human activities can also play a dominant role in regulating fire behaviour effectively through better fire management practices. In Northern Australia, indigenous fire managers use prescribed burns during the early dry season to prevent large late dry season fires, which shifts the overall temporal distribution of fire activity earlier during the primary biomass burning season. This increasing trend of prescribed burns has helped to significantly reduce the size and extent of the intense late dry season fires, indicating that such fire management practices can be effective at managing wildfires in savannas. Biomass burning can emit many chemical species that have an impact on human health. One of the most abundant and widely measured is carbon monoxide (CO), whose long-term exposure can lead to potential human health risk. CO is also a good proxy for emissions of other shorter-lived and harder-to-measure atmospheric constituents. This study is focussed on understanding how the earlier fire season in Northern Australia impacts the temporal shift in annual cycle of CO. Column CO data from the ground-based Total Carbon Column Observing Network site in Darwin will be used together with surface measurements, complemented by the surface mixing ratio observations from MOPITT, in order to disentangle the CO emitted from the study region from that measured in the column from remote emissions coupled with long-range transport. GEOS-Chem CO tagged tracer modelling capability will be used to better understand the effect of local fire emissions on the surface and column CO.

Dongxu Yang

and 30 more

TanSat is the 1st Chinese carbon dioxide (CO) measurement satellite, launched in 2016. In this study, the University of Leicester Full Physics (UoL-FP) algorithm is implemented for TanSat nadir mode XCO retrievals. We develop a spectrum correction method to reduce the retrieval errors by the online fitting of an 8 order Fourier series. The model and a priori is developed by analyzing the solar calibration measurement. This correction provides a significant improvement to the O A band retrieval. Accordingly, we extend the previous TanSat single CO weak band retrieval to a combined O A and CO weak band retrieval. A Genetic Algorithm (GA) has been applied to determine the threshold values of post-screening filters. In total, 18.3% of the retrieved data is identified as high quality compared to the original measurements. The same quality control parameters have been used in a footprint independent multiple linear regression bias correction due to the stronger correlation with the XCO retrieval error. Twenty sites of the Total Column Carbon Observing Network (TCCON) have been selected to validate our new approach for the TanSat XCO retrieval. We show that our new approach produces a significant improvement on the XCO retrieval accuracy and precision when compared to TCCON with an average bias and RMSE of -0.08 ppm and 1.47 ppm, respectively. The methods used in this study can help to improve the XCO retrieval from TanSat and subsequently the Level-2 data production, and hence will be applied in the TanSat operational XCO processing.