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Jason R. Green edited Abstract.tex
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To Fluctuating rate coefficients are necessary to describe disordered kinetic processes with phenomenological, mass-action rate
laws it is necessary to introduce fluctuating rate coefficients. laws. First-order rate laws for irreversible decay have been the primary focus of this approach, but
higher-order kinetics disorder may also
be disordered. manifest in higher-order kinetic processes. Here we present
theory for disordered a measure of the static or dynamic disorder in irreversible decay for $A^n\to \textrm{products}$, $n=1,2,3,\ldots$.
The central result is a This measure
of quantifies the cumulative deviations of the rate coefficient history from a constant value -- the inequality between the square of the time-integrated rate coefficient and the time-integrated rate coefficient squared. Application of this theory to empirical models for disordered kinetics shows this inequality measures the variation in rate coefficients for this class of kinetic processes. Traditional kinetics is valid only when the equality holds.