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We present a cloud-based analysis of the molecular gas in M83 as observed by ALMA. We compare the results of the cloud decomposition to the properties of the cluster population, searching for a connection between the structural organization of the molecular gas and the changing cluster properties. Based on this analysis, we reach the following conclusions:  \begin{enumerate}  \item The molecular clouds in M83 are well-resolved in the ALMA data and show excellent correspondence with scaling relations seen in other systems. On average, they are consistent with significant self-gravitation and a turbulence driven size-line width relationship.  \item Despite the overall correspondence between the molecular cloud populations and the scalings seen in other systems, there are systematic variations in cloud properties over the face of the galaxy. Of note, the clouds found in the nuclear region ($R_g<0.5$~kpc) have significantly higher surface densities ($\langle \Sigma \rangle = 1100 M_{\odot}~\mbox{pc}^{-2}$ vs. $300 M_{\odot}~\mbox{pc}^{-2}$ in the disk) and turbulent line widths on 1 pc scales $\langle \sigma_0\rangle = \langle \sigma_v R^{-0.5}\rangle R_0^{-0.5}\rangle  = 1.7 \mbox{ km s}^{-1}$ vs $0.7 \mbox{ km s}^{-1}$ in the disk. Despite higher densities and more intense turbulence, the clouds still have graviational binding energies comparable to their internal kinetic energies as evidenced by virial-theorem-based estimates for their mass being consistent with estimates from their CO luminosity (i.e., the $X$-factor). \item The mass distributions of molecular clouds change over the face of the galaxy. There is good evidence for a characteristic truncation mass in the population, which sets an upper limit for molecular cloud mass. Functional fits to the mass distribution are consistent with this conclusion but do not appear to reproduce the full behavior of the mass distribution. The maximum mass in the population is highest in the center of the galaxy though blending of emission features likely biases this result. Outside of the nucleus, the maximum mass cloud found in bins of equal area decreases by a factor of 5.   \item Characteristic masses have been previously observed in the cluster population and fit with a Schechter function, namely a power-law mass distribution with an exponential cutoff above a characteristic mass. There is not good evidence for this being the best representation of the molecular cloud mass distribution, but the maximum mass GMC corresponds well to the maximum mass cluster in each radial bin. Over this range the cluster and cloud masses decrease by a factor of 5.   \item Maximum cloud masses also agree reasonably well with the predictions from the Toomre criterion, which is the mass scale on which structures will form in a shearing disk. They do not agree with a strict Jeans analysis, highlighting the importance of galactic dynamical environment in shaping the resulting molecular cloud population.