Shyno Susan John

and 3 more

Fire is an essential global phenomenon that existed soon after the appearance of terrestrial plants and is vital for the regeneration of the plant species. Human activities have contributed to a changing climate and impacted fire regimes, resulting in more intense, frequent and severe fires. In particular, the 2019-20 bushfires in south-eastern Australia were unprecedented in their extent and intensity. However, human activities can also play a dominant role in regulating fire behaviour effectively through better fire management practices. In Northern Australia, indigenous fire managers use prescribed burns during the early dry season to prevent large late dry season fires, which shifts the overall temporal distribution of fire activity earlier during the primary biomass burning season. This increasing trend of prescribed burns has helped to significantly reduce the size and extent of the intense late dry season fires, indicating that such fire management practices can be effective at managing wildfires in savannas. Biomass burning can emit many chemical species that have an impact on human health. One of the most abundant and widely measured is carbon monoxide (CO), whose long-term exposure can lead to potential human health risk. CO is also a good proxy for emissions of other shorter-lived and harder-to-measure atmospheric constituents. This study is focussed on understanding how the earlier fire season in Northern Australia impacts the temporal shift in annual cycle of CO. Column CO data from the ground-based Total Carbon Column Observing Network site in Darwin will be used together with surface measurements, complemented by the surface mixing ratio observations from MOPITT, in order to disentangle the CO emitted from the study region from that measured in the column from remote emissions coupled with long-range transport. GEOS-Chem CO tagged tracer modelling capability will be used to better understand the effect of local fire emissions on the surface and column CO.
Australian fires are a primary driver of variability in Australian atmospheric composition and contribute significantly to regional and global carbon budgets. However, biomass burning emissions from Australia remain highly uncertain. In this work, we use surface in situ, ground-based total column and satellite total column observations to evaluate the ability of two global models (GEOS-Chem and ACCESS-UKCA) and three global biomass burning emission inventories (FINN1.5, GFED4s, and QFED2.4) to simulate carbon monoxide (CO) in the Australian atmosphere. We find that emissions from northern Australia savanna fires are substantially lower in FINN1.5 than in the other inventories. Model simulations driven by FINN1.5 are unable to reproduce either the magnitude or the variability of observed CO in northern Australia. The remaining two inventories perform similarly in reproducing the observed variability, although the larger emissions in QFED2.4 combined with an existing high bias in the southern hemisphere background lead to large CO biases. We therefore recommend GFED4s as the best option of the three for global modelling studies with focus on Australia or the southern hemisphere. Near fresh fire emissions, the higher resolution ACCESS-UKCA model is better able to simulate surface CO than GEOS-Chem, while GEOS-Chem captures more of the observed variability in the total column and remote surface air measurements. We also show that existing observations in Australia can only partially constrain global model estimates of biomass burning. Continuous measurements in fire-prone parts of Australia are needed, along with updates to global biomass burning inventories that are validated with Australian data.

Yang Dongxu

and 30 more

TanSat is the 1st Chinese carbon dioxide (CO) measurement satellite, launched in 2016. In this study, the University of Leicester Full Physics (UoL-FP) algorithm is implemented for TanSat nadir mode XCO retrievals. We develop a spectrum correction method to reduce the retrieval errors by the online fitting of an 8 order Fourier series. The model and a priori is developed by analyzing the solar calibration measurement. This correction provides a significant improvement to the O A band retrieval. Accordingly, we extend the previous TanSat single CO weak band retrieval to a combined O A and CO weak band retrieval. A Genetic Algorithm (GA) has been applied to determine the threshold values of post-screening filters. In total, 18.3% of the retrieved data is identified as high quality compared to the original measurements. The same quality control parameters have been used in a footprint independent multiple linear regression bias correction due to the stronger correlation with the XCO retrieval error. Twenty sites of the Total Column Carbon Observing Network (TCCON) have been selected to validate our new approach for the TanSat XCO retrieval. We show that our new approach produces a significant improvement on the XCO retrieval accuracy and precision when compared to TCCON with an average bias and RMSE of -0.08 ppm and 1.47 ppm, respectively. The methods used in this study can help to improve the XCO retrieval from TanSat and subsequently the Level-2 data production, and hence will be applied in the TanSat operational XCO processing.